Dato' Harun joined the Royal Malaysian Police (RMP) on 1 June 1970 as a Probationary Inspector. He served the RMP for 39 years and retired on 9 April 2009 with the rank of Deputy Commissioner of Police (DCP). His last post was as the Deputy Director 1, Special Branch. In his long and distinguished career with the RMP, Dato Harun had served in various capacities including as the head of Special Branch of Perak, Kedah and Sarawak.
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